Ozone profile climatology for remote sensing retrieval algorithms

Yang, Kai; Liu, Xiong

New ozone (inline-formulaO3) profile climatologies are created from the Modern-Era Retrospective Analysis for Research and Applications version 2 (MERRA-2) inline-formulaO3 record between 2005 and 2016, within the period of Aura Microwave Limb Sounder (MLS) and Aura Ozone Monitoring Instrument (OMI) assimilation. These two climatologies consist of monthly mean inline-formulaO3 profiles and the corresponding covariances dependent on the local solar time, longitude (15inline-formula), and latitude (10inline-formula), which are parameterized by tropopause pressure and total inline-formulaO3 column. They are validated through comparisons, which show good agreements with previous inline-formulaO3 profile climatologies. Compared to a monthly zonal mean climatology, both tropopause- and column-dependent climatologies provide improved a priori information for profile and total inline-formulaO3 retrievals from remote sensing measurements. Furthermore, parameterization of the inline-formulaO3 profile with total column inline-formulaO3 usually reduces the natural variability of the resulting climatological profile in the upper stratosphere further than the tropopause parameterization, which usually performs better in the upper troposphere and lower stratosphere (UTLS). Therefore tropopause-dependent climatology is more appropriate for profile inline-formulaO3 retrieval for complementing the vertical resolution of backscattered ultraviolet (UV) spectra, while the column-dependent climatology is more suited for use in total inline-formulaO3 retrieval algorithms, with an advantage of complete profile specification without requiring ancillary information. Compared to previous column-dependent climatologies, the new MERRA-2 column-dependent climatology better captures the diurnal, seasonal, and spatial variations and dynamical changes in inline-formulaO3 profiles with higher resolutions in inline-formulaO3, latitude, longitude, and season. The new MERRA-2 climatologies contain the first quantitative characterization of inline-formulaO3 profile covariances, which facilitate a new approach to improve inline-formulaO3 profiles using the most probable patterns of profile adjustments represented by the empirical orthogonal functions (EOFs) of the covariance matrices. The MERRA-2 daytime column-dependent climatology is used in the combo inline-formulaO3 and inline-formulaSO2 algorithm for retrieval from the Earth Polychromatic Imaging Camera (EPIC) on board the Deep Space Climate Observatory (DSCOVR) satellite, the Ozone Mapping and Profiler Suite Nadir Mapper (OMPS-NM) on the Suomi National Polar Partnership (SNPP), and the Ozone Monitoring Instrument (OMI) on the Aura spacecraft.

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Yang, Kai / Liu, Xiong: Ozone profile climatology for remote sensing retrieval algorithms. 2019. Copernicus Publications.

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Rechteinhaber: Kai Yang

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